Start

28/09/2023

End

31/12/2025

Status

In progress

NO LIMITHz

Start

28/09/2023

End

31/12/2025

Status

In progress

NO LIMITHz

NOnlinear LIthium niobate Metasurfaces for Integrated THz generation


The terahertz (THz) band of the electromagnetic spectrum (0.1 – 10 THz) is currently attracting massive interest due to its incredible application richness. Among others, the THz band is a key region where most of the fundamental vibrational resonances of condensed matter and proteins can be found. The utmost relevance of this strategic spectral window in fundamental physics and biology dramatically boosted the development of THz-based technologies in the last decades. Yet, several technological challenges still prevent assessing the full THz spectral window and the development of integrated devices. As a result, to date, no intense laser-based source exists in the range of 5 – 15 THz. This new ‘THz gap’ will be a major challenge for source development in the coming years. Concurrently, integrable THz platforms are extremely appealing in view of ‘portable’ THz systems, applications to integrated photonics, and development of novel hybrid systems.

NO LIMITHz proposes a potential breakthrough in this field, by developing a new family of integrated THz broadband sources with unmatched conversion efficiencies and ad-hoc wavefront shaping by means of a disruptive platform based on an innovative artificial nonlinear optical metamaterial. NO LIMITHz is based on very recent results showing that dielectric metasurfaces – two-dimensional metamaterials – enable THz light emission with efficiencies comparable to the best nonlinear optical materials in nature, but in a sub-wavelength thickness. Furthermore, it leverages our demonstrations of functional nonlinear lithium niobate metasurfaces enabling strong enhancement and dynamic control of the nonlinear optical interactions.

We will design, fabricate, and characterize novel active dielectric metasurfaces based on lithium niobate that efficiently emit THz beams over a wide bandwidth and with a well-defined polarization state. The wavefront of the generated beam can be arbitrarily set by the geometry of the metasurface enabling, for instance, the THz output to be directly focused on a specific sample location. The new approach of NO LIMITHz will enhance the THz generation efficiency from nonlinear metasurfaces by more than three orders of magnitude compared to the state-of-the-art based on plasmonic platforms. This will allow the realization of ultracompact THz sources in the 5 – 15 THz band with improved efficiency power and extended functionalities compared to existing technologies.

Publications

Nonlinear THz Generation through Optical Rectification Enhanced by Phonon–Polaritons in Lithium Niobate Thin Films

Luca Carletti, Cormac McDonnell, Unai Arregui Leon, Davide Rocco, Marco Finazzi, Andrea Toma, Tal Ellenbogen, Giuseppe Della Valle, Michele Celebrano, and Costantino De Angelis

ACS Photonics 10, 3419-3425 (2023)

DOI: 10.1021/acsphotonics.3c00924


Far-field mapping and efficient beaming of second harmonic by a plasmonic metagrating

Verneuil, Augustin, Di Francescantonio, Agostino, Zilli, Attilio, Proust, Julien, Béal, Jérémie, Petti, Daniela, Finazzi, Marco, Celebrano, Michele and Baudrion, Anne-Laure.

Nanophotonics 13, 3609-3614 (2024)

DOI: 10.1515/nanoph-2023-0842


Intrinsic nonlinear geometric phase in SHG from zincblende crystal symmetry media

Carletti, Luca, Rocco, Davide, Vincenti, Maria Antonietta, de Ceglia, Domenico and De Angelis, Costantino

Nanophotonics 13, 3321-3326 (2024)

DOI: 10.1515/nanoph-2024-0162


Nonlinear asymmetric imaging with AlGaAs metasurface

Davide Rocco, Andrea Locatelli, Luca Carletti, Maria Antonietta Vincenti, and Costantino De Angelis,

Opt. Express 32, 11673-11680 (2024). DOI:10.1364/OE.517991


Event detection via THz generation with flat nonlinear optics

Unai Arregui Leon, Paolo Franceschini, Olga Sergaeva, Andrea Tognazzi, Davide Rocco, Luca Carletti, Domenico de Ceglia, Giuseppe Della Valle, and Costantino De Angelis,

Opt. Mater. Express 15, 307-318 (2025)

DOI: 10.1364/OME.543944


THz Field Induced Second Harmonic Generation in Epsilon Near Zero Indium Tin Oxide Thin Films

Cormac McDonnell, Luca Carletti, Maria Antonietta Vincenti, Giuseppe Della Valle, Costantino De Angelis, Michele Celebrano, and Tal Ellenbogen

Nano Letters 25, 12201-12206 (2025)

DOI: 10.1021/acs.nanolett.5c02467


Nonlinear Dielectric Metasurfaces for Terahertz Applications

Habibighahfarokhi, F.; Sergaeva, O.; Carletti, L.; Franceschini, P.; Tognazzi, A.; Locatelli, A.; Leon, U.A.; Della Valle, G.; De Angelis, C.; Rocco, D.

Photonics 12, 370 (2025)

DOI: 10.3390/photonics12040370


Research labs